Adsorption of acid-extractable organics from oil sands process-affected water onto biomass-based biochar: Metal content matters.
Identifieur interne : 001537 ( Main/Exploration ); précédent : 001536; suivant : 001538Adsorption of acid-extractable organics from oil sands process-affected water onto biomass-based biochar: Metal content matters.
Auteurs : Tazul I. Bhuiyan [Canada] ; Jin K. Tak [Canada] ; Sebastian Sessarego [Canada] ; Don Harfield [Canada] ; Josephine M. Hill [Canada]Source :
- Chemosphere [ 1879-1298 ] ; 2017.
Descripteurs français
- KwdFr :
- Acides carboxyliques (composition chimique), Adsorption (MeSH), Biomasse (MeSH), Cannabis (MeSH), Champs de pétrole et de gaz (MeSH), Charbon de bois (composition chimique), Déchets industriels (MeSH), Métaux (composition chimique), Panicum (MeSH), Pinus (MeSH), Polluants chimiques de l'eau (composition chimique), Populus (MeSH), Triticum (MeSH).
- MESH :
- composition chimique : Acides carboxyliques, Charbon de bois, Métaux, Polluants chimiques de l'eau.
- Adsorption, Biomasse, Cannabis, Champs de pétrole et de gaz, Déchets industriels, Panicum, Pinus, Populus, Triticum.
English descriptors
- KwdEn :
- MESH :
- chemical , chemistry : Carboxylic Acids, Charcoal, Metals, Water Pollutants, Chemical.
- Adsorption, Biomass, Cannabis, Industrial Waste, Oil and Gas Fields, Panicum, Pinus, Populus, Triticum.
Abstract
The impact of biochar properties on acid-extractable organics (AEO) adsorption from oil sands process-affected water (OSPW) was studied. Biochar from wheat straw with the highest ash content (14%) had the highest adsorption capacity (0.59 mg/g) followed by biochar from pulp mill sludge, switchgrass, mountain pine, hemp shives, and aspen wood. The adsorption capacity had no obvious trend with surface area, total pore volume, bulk polarity and aromaticity. The large impact of metal content was consistent with the carboxylates (i.e., naphthenate species) in the OSPW binding to the metals (mainly Al and Fe) on the carbon substrate. Although the capacity of biochar is still approximately two orders of magnitude lower than that of a commercial activated carbon, confirming the property (i.e., metal content) that most influenced AEO adsorption, may allow biochar to become competitive with activated carbon after normalizing for cost, especially if this cost includes environmental impacts.
DOI: 10.1016/j.chemosphere.2016.11.126
PubMed: 27919534
Affiliations:
Links toward previous steps (curation, corpus...)
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Bhuiyan</name><affiliation wicri:level="4"><nlm:affiliation>Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Dr. N.W., Calgary, AB T2N 1N4, Canada.</nlm:affiliation><country xml:lang="fr">Canada</country><wicri:regionArea>Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Dr. N.W., Calgary, AB T2N 1N4</wicri:regionArea><orgName type="university">Université de Calgary</orgName><placeName><settlement type="city">Calgary</settlement><region type="state">Alberta</region></placeName></affiliation></author><author><name sortKey="Tak, Jin K" sort="Tak, Jin K" uniqKey="Tak J" first="Jin K" last="Tak">Jin K. Tak</name><affiliation wicri:level="1"><nlm:affiliation>Thermochemical Processing, InnoTech Alberta, P.O. Bag 4000, Vegreville, T9C 1T4, Alberta, Canada.</nlm:affiliation><country xml:lang="fr">Canada</country><wicri:regionArea>Thermochemical Processing, InnoTech Alberta, P.O. Bag 4000, Vegreville, T9C 1T4, Alberta</wicri:regionArea><wicri:noRegion>Alberta</wicri:noRegion></affiliation></author><author><name sortKey="Sessarego, Sebastian" sort="Sessarego, Sebastian" uniqKey="Sessarego S" first="Sebastian" last="Sessarego">Sebastian Sessarego</name><affiliation wicri:level="4"><nlm:affiliation>Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Dr. N.W., Calgary, AB T2N 1N4, Canada.</nlm:affiliation><country xml:lang="fr">Canada</country><wicri:regionArea>Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Dr. N.W., Calgary, AB T2N 1N4</wicri:regionArea><orgName type="university">Université de Calgary</orgName><placeName><settlement type="city">Calgary</settlement><region type="state">Alberta</region></placeName></affiliation></author><author><name sortKey="Harfield, Don" sort="Harfield, Don" uniqKey="Harfield D" first="Don" last="Harfield">Don Harfield</name><affiliation wicri:level="1"><nlm:affiliation>Thermochemical Processing, InnoTech Alberta, P.O. 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Electronic address: jhill@ucalgary.ca.</nlm:affiliation><country xml:lang="fr">Canada</country><wicri:regionArea>Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Dr. N.W., Calgary, AB T2N 1N4</wicri:regionArea><orgName type="university">Université de Calgary</orgName><placeName><settlement type="city">Calgary</settlement><region type="state">Alberta</region></placeName></affiliation></author></analytic><series><title level="j">Chemosphere</title><idno type="eISSN">1879-1298</idno><imprint><date when="2017" type="published">2017</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Adsorption (MeSH)</term><term>Biomass (MeSH)</term><term>Cannabis (MeSH)</term><term>Carboxylic Acids (chemistry)</term><term>Charcoal (chemistry)</term><term>Industrial Waste (MeSH)</term><term>Metals (chemistry)</term><term>Oil and Gas Fields (MeSH)</term><term>Panicum (MeSH)</term><term>Pinus (MeSH)</term><term>Populus (MeSH)</term><term>Triticum (MeSH)</term><term>Water Pollutants, Chemical (chemistry)</term></keywords><keywords scheme="KwdFr" xml:lang="fr"><term>Acides carboxyliques (composition chimique)</term><term>Adsorption (MeSH)</term><term>Biomasse (MeSH)</term><term>Cannabis (MeSH)</term><term>Champs de pétrole et de gaz (MeSH)</term><term>Charbon de bois (composition chimique)</term><term>Déchets industriels (MeSH)</term><term>Métaux (composition chimique)</term><term>Panicum (MeSH)</term><term>Pinus (MeSH)</term><term>Polluants chimiques de l'eau (composition chimique)</term><term>Populus (MeSH)</term><term>Triticum (MeSH)</term></keywords><keywords scheme="MESH" type="chemical" qualifier="chemistry" xml:lang="en"><term>Carboxylic Acids</term><term>Charcoal</term><term>Metals</term><term>Water Pollutants, Chemical</term></keywords><keywords scheme="MESH" qualifier="composition chimique" xml:lang="fr"><term>Acides carboxyliques</term><term>Charbon de bois</term><term>Métaux</term><term>Polluants chimiques de l'eau</term></keywords><keywords scheme="MESH" xml:lang="en"><term>Adsorption</term><term>Biomass</term><term>Cannabis</term><term>Industrial Waste</term><term>Oil and Gas Fields</term><term>Panicum</term><term>Pinus</term><term>Populus</term><term>Triticum</term></keywords><keywords scheme="MESH" xml:lang="fr"><term>Adsorption</term><term>Biomasse</term><term>Cannabis</term><term>Champs de pétrole et de gaz</term><term>Déchets industriels</term><term>Panicum</term><term>Pinus</term><term>Populus</term><term>Triticum</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">The impact of biochar properties on acid-extractable organics (AEO) adsorption from oil sands process-affected water (OSPW) was studied. Biochar from wheat straw with the highest ash content (14%) had the highest adsorption capacity (0.59 mg/g) followed by biochar from pulp mill sludge, switchgrass, mountain pine, hemp shives, and aspen wood. The adsorption capacity had no obvious trend with surface area, total pore volume, bulk polarity and aromaticity. The large impact of metal content was consistent with the carboxylates (i.e., naphthenate species) in the OSPW binding to the metals (mainly Al and Fe) on the carbon substrate. Although the capacity of biochar is still approximately two orders of magnitude lower than that of a commercial activated carbon, confirming the property (i.e., metal content) that most influenced AEO adsorption, may allow biochar to become competitive with activated carbon after normalizing for cost, especially if this cost includes environmental impacts.</div></front></TEI><pubmed><MedlineCitation Status="MEDLINE" IndexingMethod="Curated" Owner="NLM"><PMID Version="1">27919534</PMID><DateCompleted><Year>2017</Year><Month>01</Month><Day>27</Day></DateCompleted><DateRevised><Year>2018</Year><Month>12</Month><Day>02</Day></DateRevised><Article PubModel="Print-Electronic"><Journal><ISSN IssnType="Electronic">1879-1298</ISSN><JournalIssue CitedMedium="Internet"><Volume>168</Volume><PubDate><Year>2017</Year><Month>Feb</Month></PubDate></JournalIssue><Title>Chemosphere</Title><ISOAbbreviation>Chemosphere</ISOAbbreviation></Journal><ArticleTitle>Adsorption of acid-extractable organics from oil sands process-affected water onto biomass-based biochar: Metal content matters.</ArticleTitle><Pagination><MedlinePgn>1337-1344</MedlinePgn></Pagination><ELocationID EIdType="pii" ValidYN="Y">S0045-6535(16)31669-1</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.1016/j.chemosphere.2016.11.126</ELocationID><Abstract><AbstractText>The impact of biochar properties on acid-extractable organics (AEO) adsorption from oil sands process-affected water (OSPW) was studied. Biochar from wheat straw with the highest ash content (14%) had the highest adsorption capacity (0.59 mg/g) followed by biochar from pulp mill sludge, switchgrass, mountain pine, hemp shives, and aspen wood. The adsorption capacity had no obvious trend with surface area, total pore volume, bulk polarity and aromaticity. The large impact of metal content was consistent with the carboxylates (i.e., naphthenate species) in the OSPW binding to the metals (mainly Al and Fe) on the carbon substrate. Although the capacity of biochar is still approximately two orders of magnitude lower than that of a commercial activated carbon, confirming the property (i.e., metal content) that most influenced AEO adsorption, may allow biochar to become competitive with activated carbon after normalizing for cost, especially if this cost includes environmental impacts.</AbstractText><CopyrightInformation>Copyright © 2016 Elsevier Ltd. All rights reserved.</CopyrightInformation></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Bhuiyan</LastName><ForeName>Tazul I</ForeName><Initials>TI</Initials><AffiliationInfo><Affiliation>Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Dr. N.W., Calgary, AB T2N 1N4, Canada.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Tak</LastName><ForeName>Jin K</ForeName><Initials>JK</Initials><AffiliationInfo><Affiliation>Thermochemical Processing, InnoTech Alberta, P.O. Bag 4000, Vegreville, T9C 1T4, Alberta, Canada.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Sessarego</LastName><ForeName>Sebastian</ForeName><Initials>S</Initials><AffiliationInfo><Affiliation>Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Dr. N.W., Calgary, AB T2N 1N4, Canada.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Harfield</LastName><ForeName>Don</ForeName><Initials>D</Initials><AffiliationInfo><Affiliation>Thermochemical Processing, InnoTech Alberta, P.O. Bag 4000, Vegreville, T9C 1T4, Alberta, Canada.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Hill</LastName><ForeName>Josephine M</ForeName><Initials>JM</Initials><AffiliationInfo><Affiliation>Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Dr. N.W., Calgary, AB T2N 1N4, Canada. Electronic address: jhill@ucalgary.ca.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2016</Year><Month>12</Month><Day>03</Day></ArticleDate></Article><MedlineJournalInfo><Country>England</Country><MedlineTA>Chemosphere</MedlineTA><NlmUniqueID>0320657</NlmUniqueID><ISSNLinking>0045-6535</ISSNLinking></MedlineJournalInfo><ChemicalList><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D002264">Carboxylic Acids</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D007220">Industrial Waste</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D008670">Metals</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="D014874">Water Pollutants, Chemical</NameOfSubstance></Chemical><Chemical><RegistryNumber>0</RegistryNumber><NameOfSubstance UI="C540010">biochar</NameOfSubstance></Chemical><Chemical><RegistryNumber>16291-96-6</RegistryNumber><NameOfSubstance UI="D002606">Charcoal</NameOfSubstance></Chemical></ChemicalList><CitationSubset>IM</CitationSubset><MeshHeadingList><MeshHeading><DescriptorName UI="D000327" MajorTopicYN="N">Adsorption</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D018533" MajorTopicYN="N">Biomass</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D002188" MajorTopicYN="N">Cannabis</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D002264" MajorTopicYN="N">Carboxylic Acids</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="N">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D002606" MajorTopicYN="N">Charcoal</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D007220" MajorTopicYN="N">Industrial Waste</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D008670" MajorTopicYN="N">Metals</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading><MeshHeading><DescriptorName UI="D061329" MajorTopicYN="Y">Oil and Gas Fields</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D008897" MajorTopicYN="N">Panicum</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D028223" MajorTopicYN="N">Pinus</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D032107" MajorTopicYN="N">Populus</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D014908" MajorTopicYN="N">Triticum</DescriptorName></MeshHeading><MeshHeading><DescriptorName UI="D014874" MajorTopicYN="N">Water Pollutants, Chemical</DescriptorName><QualifierName UI="Q000737" MajorTopicYN="Y">chemistry</QualifierName></MeshHeading></MeshHeadingList><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Acid-extractable organics</Keyword><Keyword MajorTopicYN="N">Adsorption</Keyword><Keyword MajorTopicYN="N">Biochar</Keyword><Keyword MajorTopicYN="N">Naphthenic acids</Keyword><Keyword MajorTopicYN="N">Oil sands process-affected water</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2016</Year><Month>08</Month><Day>30</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2016</Year><Month>11</Month><Day>24</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2016</Year><Month>11</Month><Day>25</Day></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2016</Year><Month>12</Month><Day>7</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2017</Year><Month>1</Month><Day>28</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2016</Year><Month>12</Month><Day>7</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate></History><PublicationStatus>ppublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">27919534</ArticleId><ArticleId IdType="pii">S0045-6535(16)31669-1</ArticleId><ArticleId IdType="doi">10.1016/j.chemosphere.2016.11.126</ArticleId></ArticleIdList></PubmedData></pubmed><affiliations><list><country><li>Canada</li></country><region><li>Alberta</li></region><settlement><li>Calgary</li></settlement><orgName><li>Université de Calgary</li></orgName></list><tree><country name="Canada"><region name="Alberta"><name sortKey="Bhuiyan, Tazul I" sort="Bhuiyan, Tazul I" uniqKey="Bhuiyan T" first="Tazul I" last="Bhuiyan">Tazul I. Bhuiyan</name></region><name sortKey="Harfield, Don" sort="Harfield, Don" uniqKey="Harfield D" first="Don" last="Harfield">Don Harfield</name><name sortKey="Hill, Josephine M" sort="Hill, Josephine M" uniqKey="Hill J" first="Josephine M" last="Hill">Josephine M. Hill</name><name sortKey="Sessarego, Sebastian" sort="Sessarego, Sebastian" uniqKey="Sessarego S" first="Sebastian" last="Sessarego">Sebastian Sessarego</name><name sortKey="Tak, Jin K" sort="Tak, Jin K" uniqKey="Tak J" first="Jin K" last="Tak">Jin K. Tak</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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